Popsugar Entertainment Disney Movies Toy Story 4 Cast The Entire Toy Story 4 Cast, From Old Favourites to Brand-New Characters 14 November 2018 by Quinn Keaney View On One Page Photo 11 of 14 ADVERTISEMENT () Start Slideshow Share This Link Copy ← Use Arrow Keys → 11 Jeff Garlin as Buttercup Has there ever been a more surprising combination of voice and character than Jeff Garlin's Buttercup? Previous Next Start Slideshow Disney MoviesToy Story 4Movie CastingMovies